Background: Polyethylene composites including boron can be used as an effective neutron shield. Our investigation focuses on manufacturing borated polyethylene nano-composite. The purpose of this study is to design a radiation shield for use in both neutron and gamma fields. Materials and Methods: Borated polyethylene shields containing 2%, and 5% weight percentage of Boron nano-particles were constructed and their neutron attenuation was compared with pure polyethylene. Polycarbonate films were used to find the attenuation of Am-Be neutrons after passing the shields. Mechanical properties of the shields were finally compared. Results: Mean  (± SD) number of α tracks induced by neutrons passing through the shields, were found to be 1.0488×10³±128.98,  1.1972×10³±289.56and 1.5340×10³±206.52 for polyethylene with 5% by weight, polyethylene with 2% by weight boron nano-particles, and pure polyethylene, respectively. The neutron spectrum after each shield was also obtained by MCNP4C Monte Carlo simulations. On the other hand, borated polyethylene nano-composites showed higher tensile strength compared to that of pure polyethylene. Attenuation of neutrons measured in experiments and the result of MCNP simulation were in good agreement. Conclusion: A statistically significant difference was found between neutron attenuation by borated polyethylene nanocomposite made of 5% by weight boron and pure polyethylene. However, the difference between borated polyethylene nano-composite with 5% weight and 2% wt boron was not statistically significant.